Advances in Chemical Physics, by Stuart A. Rice

By Stuart A. Rice

This sequence offers the chemical physics box with a discussion board for serious, authoritative reviews of advances in each zone of the self-discipline. This stand-alone targeted subject matters quantity reviews fresh advances in electron-transfer learn with major, up to date chapters through the world over well-known researchers.

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Chem. Phys. 124, 224316 (2006). OPTIMAL CONTROL THEORY FOR MANIPULATING MOLECULAR PROCESSES GABRIEL G. BALINT-KURTI and SHIYANG ZOU School of Chemistry, University of Bristol, Bristol BS8 1TS, UK ALEX BROWN Department of Chemistry, University of Alberta, Edmonton, AB, T6G 2G2, Canada CONTENTS I. Introduction II. Optimal Control Theory A. Basic Formalism B. Additional Restrictions on Laser Pulse C. Photodissociation III. Methods for Solving the Optimal Control Problem A. Conjugate Gradient Method B.

If this route passes by one or more exit channels then the path is looping; if it does not, then the path is direct. It is then clear that the GP changes the sign of the direct reactive with respect to the direct inelastic contribution, and that it leaves unchanged the sign of the looping reactive with respect to the direct inelastic. The first of these observations is Mead’s result [14]; the second is the required generalization of Mead’s result to an encircling nuclear wave function. Although we have considered here a reaction that has the same particle-exchange symmetry as the H þ H2 reaction, the arguments above can clearly be generalized to treat reactions of any symmetry.

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